Hyperpolarisability of (donor)2‐acceptor‐type molecules determined by EFISHG
作者:
Isabelle Maltey,
Jacques A. Delaire,
Keitaro Nakatani,
Pengfei Wang,
Xiangyang Shi,
Shikang Wu,
期刊:
Advanced Materials for Optics and Electronics
(WILEY Available online 1996)
卷期:
Volume 6,
issue 5‐6
页码: 233-238
ISSN:1057-9257
年代: 1996
DOI:10.1002/(SICI)1099-0712(199609)6:5/6<233::AID-AMO272>3.0.CO;2-1
出版商: John Wiley&Sons Ltd.
关键词: non‐linear optics;EFISHG;and‐shaped molecules;hyperporisability
数据来源: WILEY
摘要:
AbstractMolecular first‐order hyperpolarisabilities β of (donor)2‐acceptor type molecules have been determined by electric field induced second‐harmonic generation (EFISHG) experiments at 1.06 μm. The hyperpolarisability values are enhanced in these two dimensional charge transfer molecules, compared with a reference linear model molecule. One of these molecules absorbs part of the second‐harmonic beam. We propose a determination method for β that takes into account this phenomenon. Crystals of the title molecules exhibit second harmonic generation by the p
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