Molecular Orientation, Pair Correlations and Cascading in Nonlinear Optical Susceptibilties
作者:
JamesH. Andrews,
KennethL. Kowalski,
KennethD. Singer,
期刊:
Molecular Crystals and Liquid Crystals Science and Technology. Section A. Molecular Crystals and Liquid Crystals
(Taylor Available online 1992)
卷期:
Volume 223,
issue 1
页码: 143-150
ISSN:1058-725X
年代: 1992
DOI:10.1080/15421409208048247
出版商: Taylor & Francis Group
数据来源: Taylor
摘要:
Different susceptibility expansions for the polarization densityPare compared to identify cascading contributions to the nonlinear response of a medium. In certain liquids pair-correlation dependence of the nonlinear optical susceptibilities has been observed. To isolate the cascading effects that depend most sensitively on pair correlation and near-field effects, a simple statistical model forPis applied to the case of a liquid whose oriented molecules have only first hyperpolarizabilities; then all third-order effects inPare a consequence of cascading.
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