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Single molecule fluorescence in inhomogeneous environments

 

作者: Lukas Novotny,  

 

期刊: Applied Physics Letters  (AIP Available online 1996)
卷期: Volume 69, issue 25  

页码: 3806-3808

 

ISSN:0003-6951

 

年代: 1996

 

DOI:10.1063/1.117111

 

出版商: AIP

 

数据来源: AIP

 

摘要:

A single molecule in an inhomogeneous environment is studied theoretically using phenomenological theory. The molecule is located on a planar glass substrate and a finite sized, three dimensional object is scanned over the molecule at different heights. Lifetime and quantum yield are calculated as a function of the lateral position of the object. The analysis is based on a new field expansion method using Green’s functions of a layered reference system as basis functions. It is found that, near the edges of the object, the molecular lifetime is highly sensitive to the orientation of the transition dipole. ©1996 American Institute of Physics.

 

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