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CATALYTIC COMBUSTION OF NATURAL GAS IN A FIXED BED REACTOR WITH FLOW REVERSAL

 

作者: C. SAPUNDZHIEV,   J. CHAOUKI,   C. GUY,   D. KLVANA,  

 

期刊: Chemical Engineering Communications  (Taylor Available online 1993)
卷期: Volume 125, issue 1  

页码: 171-186

 

ISSN:0098-6445

 

年代: 1993

 

DOI:10.1080/00986449308936201

 

出版商: Taylor & Francis Group

 

关键词: Fixed bed flow reversal reactor;Catalytic combustion;No-NOxcombustion

 

数据来源: Taylor

 

摘要:

A new application of the fixed bed catalytic reactor with flow reversal for combustion of natural gas is investigated by mathematical modeling and computer simulation. Comparison between the results obtained for this new reactor and those for a classic catalytic fixed bed is made. Inexpensive perovskite type catalysts containing no noble metals were used. It is shown that an appropriate choice of operating parameters (concentration and temperature of input gas mixture, superficial gas velocity, size and shape of catalyst and inert material, volumetric ratio between catalyst and inert material in the bed) allows for a methane combustion at must lower temperatures in the reactor with flow reversal than in a classic catalytic reactor. Under such a low temperature combustion, no nitrogen oxides are produced.

 

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