Simulation of collision-induced absorption spectra rare-gas gaseous mixtures including ternary effects
作者:
Shmuel Weiss,
期刊:
Molecular Physics
(Taylor Available online 1990)
卷期:
Volume 71,
issue 3
页码: 623-634
ISSN:0026-8976
年代: 1990
DOI:10.1080/00268979000102011
出版商: Taylor & Francis Group
数据来源: Taylor
摘要:
Simulations of rare-gas gaseous mixtures taking ternary interactions into account are performed. Simulations include Ne-Ar-Kr at 300 K and He-Ar, with Ar in excess, at 165 K. The He-Ar mixtures, which were studied in more detail, give rise to a collision-induced absorption spectrum with a well-formed dip at zero frequency. The dip becomes discernible at a Ar density of 132 amagat when the ternary contribution to the zeroth moment amounts to only 2%. Interactions are assumed to be pairwise-additive.
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