Viscoelastic response of electrorheological fluids. I. Frequency dependence
作者:
T. C. B. McLeish,
T. Jordan,
M. T. Shaw,
期刊:
Journal of Rheology
(AIP Available online 1991)
卷期:
Volume 35,
issue 3
页码: 427-448
ISSN:0148-6055
年代: 1991
DOI:10.1122/1.550222
出版商: The Society of Rheology
关键词: Electrorheology;Viscoelasticity;Suspensions;Particle–string models;FREQUENCY DEPENDENCE;ELECTROHYDRODYNAMICS;POLYMERS;STRESSES
数据来源: AIP
摘要:
We calculate the linear frequency‐dependent modulus of a model electrorheological (ER) fluid at low and intermediate concentrations, assuming that particle strings are the dominant structures. At low concentrations hydrodynamic interactions along a single string act to reduce the dissipation of modes with low wave number (just as in the case of random‐coil polymers). At higher concentrations we expect hydrodynamic screening to be effective. This results in a dissipative part to the modulus.G ‘(ω) which has a broad plateau over a frequency bandwidth (L/a)2, whereLis the characteristic string length andaof the order of the particle size. By contrast, the magnitude ofG ‘(ω) is limited by the fraction of incomplete or broken strings. The real part of the dynamic modulusG ’(ω) is dominated by strings which span the electrodes, and shows very little structure with frequency when the majority of strings are complete.
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