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Extending a continuous scan Fourier transform spectrometer for time-resolved Fourier transform spectroscopy with<0.5 cm−1spectral and<10 nstime resolution in the visible region

 

作者: Jo¨rg Lindner,   Oliver Stahlhut,   Ralf Wilhelm,   Karsten Ermisch,  

 

期刊: Review of Scientific Instruments  (AIP Available online 1998)
卷期: Volume 69, issue 4  

页码: 1629-1636

 

ISSN:0034-6748

 

年代: 1998

 

DOI:10.1063/1.1148819

 

出版商: AIP

 

数据来源: AIP

 

摘要:

The extension of a continuous scan high spectral resolution(0.006 cm−1)Fourier transform spectrometer for time-resolved Fourier transform spectroscopy with a temporal resolution in the ns regime is described. The time resolution is achieved by synchronizing a laser/transient digitizer system with the interferometer. The realization of the data acquisition and the experimental setup are described. Examples of time-resolved measurements are given. Detector limited temporal resolution of<10 nsis shown by recording scattered light from a pulsed dye laser. Spectral resolution of<0.5 cm−1is demonstrated by observing the fluorescence of electronically excited CH radicals produced in the multi photon dissociation ofCHBr3.The signal-to-noise behavior of time-resolved Fourier transform apparatus is investigated as a function of spectral (0.1–4.0 cm−1unapodized) and time resolution and of the intensity of the detected light. ©1998 American Institute of Physics.

 

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