Phase modulation technique for eliminating phase noise in picosecondT2measurements based on stimulated Raman gain
作者:
Martine De Mazie`re,
Dirk Schoemaker,
期刊:
Journal of Applied Physics
(AIP Available online 1985)
卷期:
Volume 58,
issue 4
页码: 1439-1449
ISSN:0021-8979
年代: 1985
DOI:10.1063/1.336073
出版商: AIP
数据来源: AIP
摘要:
The pump and probe variant of the stimulated Raman gain technique permits the measurement of picosecond dephasing times with low‐power, continuous‐wave mode‐locked lasers, but it suffers by its susceptibility to inevitable randomly induced fluctuations in the relative phases of the interacting laser fields. The resulting severe requirements on optical stability can be circumvented through application of a double‐modulation–detection scheme that we have developed. It is based on rms detection of theT2signal as generated through application of a low‐frequency phase modulation of precise amplitude, additional to the commonly applied rf modulation with corresponding lock‐in detection. A detailed description of the method and its experimental realization is presented.T2measurements on the 656 cm−1vibration of liquid CS2illustrate its performance. In comparison with previous techniques, precision is improved by about a factor of 4. But more important is the fact that the technique permits to make a continuous recording of theT2signal, while achieving at the same time a reduction in measurement time by an order of magnitude. Furthermore, optimization of the optical setup is possible, through direct monitoring of the dephasing signal at any delay. Automating the data taking and processing should be straightforward.
点击下载:
PDF
(927KB)
返 回