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EXPERIMENTAL AND MODELING STUDIES OF STAGED COMBUSTION USING A REACTOR ENGINEERING APPROACH

 

作者: FUHE MAO,   ROBERTB. BARAT,  

 

期刊: Chemical Engineering Communications  (Taylor Available online 1996)
卷期: Volume 145, issue 1  

页码: 1-21

 

ISSN:0098-6445

 

年代: 1996

 

DOI:10.1080/00986449608936465

 

出版商: Taylor & Francis Group

 

关键词: Experimental;Modeling;Combustion;Reaction engineering

 

数据来源: Taylor

 

摘要:

Combustion research, long dominated by mechanical engineers, is becoming increasingly a chemical engineering application. It is therefore desirable to have a well defined reactor in which to conduct combustion chemistry studies. A two zone laboratory reactor emulating a perfectly stirred reactor + plug flow reactor (PSR + PFR) sequence has been constructed and validated for use in high temperature normal and staged combustion studies. A premixed fuel/eed enters the backmixed primary zone. The effluent mixes with additional injected oxidant and/or steam, and then enters the linear flow secondary zone. Extracted gas samples from cooled probes located in each zone are subjected to several dedicated on-line stack gas analyzers, and separation/analyses by on-line gas chromatography. Detailed reaction mechanisms from the literature are incorporated into a PSR + PFR reactor engineering model. The experimental feed rates and measured temperatures are also input to the model. Good comparisons between model predictions and experimental data have been obtained for normal and air-staged combustion studies. Rate-of-prod,uction calculations from the modeling offers helpful insight into the reaction pathways responsible for important species, especially pollutants.

 

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