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Fission fragment damage in zircon

 

作者: E.R. Vance,   J.N. Boland,  

 

期刊: Radiation Effects  (Taylor Available online 1975)
卷期: Volume 26, issue 3  

页码: 135-139

 

ISSN:0033-7579

 

年代: 1975

 

DOI:10.1080/00337577508234742

 

出版商: Taylor & Francis Group

 

数据来源: Taylor

 

摘要:

X-ray diffraction, electron microscope and optical studies have been : ade on zircons damaged by fission fragments derived from the action of neutrons on uranium impurities in the zircon lattice. A dosage of about 1014fission events · cm−3was required to produce diffuse x-ray scattering, observable by conventional photographic methods, and a dosage of about 1016fission events · cm−3appears to be required to render a zircon amorphous. An optical absorption band, generated apparently by γ-rays, was observed near 270 nm in undoped zircon. The valence state of the uranium impurities was unchanged by irradiation with 1014fission events · cm−3, 2 × 1018nvt of fast neutrons, or ∼1010R of γ-rays. A fission event in zircon was deduced to produce ∼104times more displacement damage than an α-recoil atom. Individual fission tracks were observed directly by electron microscopy after dosage of 1010-1013fission events - cm−3, the tracks being similar in appearance to those found by other workers in other materials. With increasing dosage, fission fragment uradiation appears to produce a progressive disordering of the lattice, as was previously deduced for the case of α-recoil irradiation, rather than the formation of new crystallographic phases.

 

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