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Low‐resistivity epitaxial YBa2Cu3O7thin films with improved microstructure and reduced microwave losses

 

作者: U. Poppe,   N. Klein,   U. Da¨hne,   H. Soltner,   C. L. Jia,   B. Kabius,   K. Urban,   A. Lubig,   K. Schmidt,   S. Hensen,   S. Orbach,   G. Mu¨ller,   H. Piel,  

 

期刊: Journal of Applied Physics  (AIP Available online 1992)
卷期: Volume 71, issue 11  

页码: 5572-5578

 

ISSN:0021-8979

 

年代: 1992

 

DOI:10.1063/1.350535

 

出版商: AIP

 

数据来源: AIP

 

摘要:

Epitaxial thin films of YBa2Cu3O7have been prepared on SrTiO3and LaAlO3substrates by a high‐pressure planar dc‐sputtering technique. By covering the substrate heater with a frame of polycrystalline YBa2Cu3O7substantial improvements of the YBa2Cu3O7film properties were achieved. These are characterized by dc‐resistivity values &rgr;(T) of less than 50 &mgr;&OHgr; cm at 100 K and &rgr;(300 K)/&rgr;(100 K) values of up to 3.9. Significant deviations from the usual linear &rgr;(T) behavior were found. Critical temperatures above 90 K, resistive transition widths down to 0.3 K, and critical current densities of about 5 × 106A/cm2at 77 K confirm the high quality of the films. As indicated by Rutherford backscattering and high‐resolution transmission electron microscopy the films exhibit a microstructure characterized by a reduced density of lattice defects. However, lattice‐coherent precipitates with a diameter of about 5–10 nm were observed. As an outstanding feature the films exhibit, besides the initial steep falloff atTc, a further gradual decrease of the microwave surface resistance at 87 GHz below 50 K by at least one order of magnitude. These results are very promising for millimeter‐wave applications of epitaxial YBa2Cu3O7thin films.

 

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