Optical Nonlinearity by Photoinduced Variation of Intermolecular Forces in Liquids and Liquid Crystals
作者:
Lorenzo Marrucci,
期刊:
Molecular Crystals and Liquid Crystals Science and Technology. Section A. Molecular Crystals and Liquid Crystals
(Taylor Available online 1998)
卷期:
Volume 321,
issue 1
页码: 57-75
ISSN:1058-725X
年代: 1998
DOI:10.1080/10587259808025076
出版商: Taylor & Francis Group
关键词: nonlinear optics;liquid crystals;dye;intermolecular forces
数据来源: Taylor
摘要:
Recent experimental and theoretical results on the optical nonlinearity associated with molecular reorientation in dye-doped liquids and liquid crystals are reviewed. The variation of intermolecular forces experienced by a photo-excited dye molecule and the resulting change of molecular-statistical parameters such as rotational friction and orientational energy appear to be at the core of this effect. Photoinduced intramolecular charge transfer could be the cause of such variation. The angular momentum conservation is also discussed.
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