we report the results of experiments on the spin-up of two layers of immiscible fluid with a free upper surface in a rotating cylinder over a wide range of internal Froude numbers. Observations of the evolution of the velocity field by particle tracking indicates that spin-up of the azimuthal velocity in the upper layer take much longer than in a homogeneous fluid. Initially, spin-up occurs at a rate comparable to that of homogeneous fluid but, at high internal Froude number, a second phase follows in which the remaining lative motion decays much more slowly. Quantitative comparison of these measurements to the theory of Pedlosky (1967) shows good agreement.