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The diels‐alder reaction and copolymerization of halogenated N‐phenylmaleimides with dienes

 

作者: Jan Lokaj,   Hana Pivcová,   František Hrabák,  

 

期刊: Die Angewandte Makromolekulare Chemie  (WILEY Available online 1986)
卷期: Volume 144, issue 1  

页码: 207-218

 

ISSN:0003-3146

 

年代: 1986

 

DOI:10.1002/apmc.1986.051440118

 

出版商: Hüthig&Wepf Verlag

 

数据来源: WILEY

 

摘要:

AbstractThe course of the Diels‐Alder reaction of N‐(2,4,6‐tri‐bromophenyl)maleimide (I) with 2‐methyl‐1,3‐butadiene (Ip) and of N‐(2,4,6‐trichlorophenyl)maleimide (II) with Ip, 2‐chloro‐1,3‐butadiene (Cp), and butadiene (Bt) in CHCl3was investigated. For the I‐Ip addition, the reaction order was determined with respect to both components, and the activation energy was calculated. The Diels‐Alder adducts thus obtained were characterized by elementary analysis, by1H‐ and13C‐NMR spectra, specific volume contractions, melting points, solubilities, and polymerization abilities. Copolymers of I and II with Ip, Cp, Bt, and 2‐methylpropene (Ib) were prepared, and their composition was determined. The copolymerization and Diels‐Alder addition of I‐Ip and II‐Ip occurring in parallel were investigated, and the participation of these two proces

 

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