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Extremely low excitation threshold, superradiant, molecular aggregate lasing system
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Extremely low excitation threshold, superradiant, molecular aggregate lasing system
作者:
Serdar O¨zc¸elik,
Daniel L. Akins,
期刊:
Applied Physics Letters
(AIP Available online 1997)
卷期:
Volume 71,
issue 21
页码: 3057-3059
ISSN:0003-6951
年代: 1997
DOI:10.1063/1.119435
出版商: AIP
数据来源: AIP
摘要:
An extremely low threshold for lasing from a specially formulated system involving self-assembled, aggregated molecules enables the system to function as a mirrorless laser. Superradiant energy states created in coherently coupled aggregated molecules emit photons that stimulate emission from other spatially distributed superradiant states. This study focuses on a cyanine dye (specifically,1,1′-3,3′-tetraethyl-5,5′,6,6′-tetrachlorobenzimidazolocarbocyanineiodide) adsorbed onto silica colloid on which the dye aggregates, forming excitonic states involving coherent domains in which a finite number of molecules act cooperatively in the process of emitting photons. It is found that lasing from such a system is induced at a threshold of ca. 39 pJ/pulse, which corresponds to a factor of3×10+4times smaller than the lowest lasing threshold reported in the literature. ©1997 American Institute of Physics.
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