Temporal heterogeneity of the slow dynamics of a colloidal paste
作者:
Pierre Ballesta,
Christian Ligoure,
Luca Cipelletti,
期刊:
AIP Conference Proceedings
(AIP Available online 1904)
卷期:
Volume 708,
issue 1
页码: 68-71
ISSN:0094-243X
年代: 1904
DOI:10.1063/1.1764063
出版商: AIP
数据来源: AIP
摘要:
We investigate the slow dynamics of a soft glass, a concentrated suspension of polydisperse colloidal particles, by using multispeckle Diffusing Wave Spectroscopy (DWS). Two distinct regimes are observed: for small sample age,tw, the dynamics smoothly slows down, as revealed by a nearly linear increase of the characteristic relaxation time, &tgr;s, measured by DWS. At longer ages, the dynamics is quasi stationary, but &tgr;sexhibit anomalously large fluctuations in time. The time scale of the dynamical fluctuations is found to be slightly shorter than the average relaxation time. The variance of the intensity correlation function is maximum for time delays comparable to the average relaxation time, in striking analogy with recent simulations of glass‐forming liquids. © 2004 American Institute of Physics
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