Stable carbon isotopic composition of methane from some natural and anthropogenic sources
作者:
Charles M. Stevens,
Antoinette Engelkemeir,
期刊:
Journal of Geophysical Research: Atmospheres
(WILEY Available online 1988)
卷期:
Volume 93,
issue D1
页码: 725-733
ISSN:0148-0227
年代: 1988
DOI:10.1029/JD093iD01p00725
数据来源: WILEY
摘要:
The results of δ13C measurements of several types of major sources of atmospheric methane are as follows: rice paddies, −67‰; the peat bogs of the Lake Agassiz region of northern Minnesota, −67±5‰; swamps of the Florida Everglades, −55±3‰ and biomass burning, −24 to −32‰. In addition, results are presented of a study of the δ13C of CH4released from a slough, compared to the CH4in the bottom sediment. These isotopic values are used, together with previously published data, to make up a tentative budget of the fluxes of the major sources for atmospheric methane with an average isotopic composition matching the measured value for atmospheric CH4, taking into account the fractionation effect of the sink processes. This budget requires the existence of a significant flux from an anthropogenic source of heavy CH4, calculated to be 45±15 Tg yr−1if attributed to CH4from biomass
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