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Electrochemical Synthesis of Deuterio Organic Compounds. I. Electrochemical Reduction of 1-Halonaphthalenes and Synthesis of 1-Chloro-4-methylnaphthalene

 

作者: Roger N. Renaud,  

 

期刊: Canadian Journal of Chemistry  (NRC Available online 1974)
卷期: Volume 52, issue 3  

页码: 376-380

 

ISSN:0008-4042

 

年代: 1974

 

DOI:10.1139/v74-060

 

出版商: NRC Research Press

 

数据来源: NRC

 

摘要:

Electrochemical reduction of 1-chloro-, 1-bromo-, 1-iodo-, 1-chloro-4-methyl-, and 1-bromo-4-methyl naphthalene was done in presence of deuterated water. The deuterium content of the naphthalene obtained reveals that the mechanism for the bromo and the iodo derivatives might involve either a simultaneous transfer of two electrons or an organometallic intermediate, while reduction of the chloro derivative might proceed at least partially via a radical intermediate.The synthesis of 1-chloro-4-methylnaphthalene from 1-chloro-4-chloromethylnaphthalene was achieved either by selective sodium borohydride reduction or by selective electrochemical reduction.

 

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