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Depolarized Light Mixing for Light Beating Spectroscopy

 

作者: Akiyoshi Wada,   Kunitsugu Soda,   Toyoichi Tanaka,   Nobuhiro Suda,  

 

期刊: Review of Scientific Instruments  (AIP Available online 1970)
卷期: Volume 41, issue 6  

页码: 845-853

 

ISSN:0034-6748

 

年代: 1970

 

DOI:10.1063/1.1684661

 

出版商: AIP

 

数据来源: AIP

 

摘要:

The depolarized light mixing (DLM) system is presented as a useful device in light beating spectroscopy for the observation of molecular rotation, deformation, and reaction which accompany an anisotropic change of polarizability. The system has the following merits: (1) Doppler broadening does not appear because it observes forward scattering; (2) only the line shape coming from a pure anisotropic polarizability change is obtained; (3) it can work automatically as an optical heterodyne system with the stray light from the second polarizer serving as a local oscillator light; (4) there is no difficulty in matching the wavefronts of the scattered light and local oscillator beam; and (5) the scattering volume can be made large without diminishing the efficiency of light beating. These characteristics are described through the numerical evaluation of beating efficiency and signal‐to‐noise ratio.

 

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