Sealed can- and alpha-autoradiography techniques were used to estimate the effective and real contents of Ra-224 respectively in Egyptian black sand samples collected from Rosetta City in the Nile Delta at the North Coast of Egypt. The effective Ra-224 content was found to be 15 ± 3 Bq · kg−1. From the average chemical composition of the black sand samples, the range-energy relation for the alpha-particles of the thorium series was calculated. Assuming radioactive equilibrium, the real Ra-224 content for samples collected from different regions were found to range from 90 to 900 Bq · kg−1. As a result, the total emanation power was measured and then used to estimate grain diameter of the black sand. The average mass exhalation rate of the different locations in Rosetta City was also estimated.